Abstract

The impact of aerosol particles on the formation and properties of clouds is one of the largest remaining sources of uncertainty in climate change projections. Certain aerosol particles, known as ice nuclei, initiate ice-crystal formation in clouds, thereby affecting precipitation and the global ... Show moreThe impact of aerosol particles on the formation and properties of clouds is one of the largest remaining sources of uncertainty in climate change projections. Certain aerosol particles, known as ice nuclei, initiate ice-crystal formation in clouds, thereby affecting precipitation and the global hydrological cycle. Laboratory studies suggest that some mineral dusts and primary biological particles-such as bacteria, pollen and fungi-can act as ice nuclei. Here we use aircraft-aerosol time-of-flight spectrometry to directly measure the chemistry of individual cloud ice-crystal residues (obtained after evaporation of the ice), which were sampled at high altitude over Wyoming. We show that biological particles and mineral dust comprised most of the ice-crystal residues: mineral dust accounted for ∼50% of the residues and biological particles for ∼33%. Along with concurrent measurements of cloud ice-crystal and ice-nuclei concentrations, these observations suggest that certain biological and dust particles initiated ice formation in the sampled clouds. Finally, we use a global aerosol model to show long-range transport of desert dust, suggesting that biological particles can enhance the impact of desert dust storms on the formation of cloud ice. Show less